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Periodic deprivation of gaseous hydrogen sulfide affects the activity of the concrete corrosion layer in sewers
Sun, Xiaoyan1,3; Jiang, Guangming1,2; Bond, Philip L.1; Keller, Jurg1
2019-06-15
Source PublicationWATER RESEARCH
ISSN0043-1354
Volume157Issue:1Pages:463-471
Abstract

Sulfide induced concrete corrosion significantly reduces the service life of the sewer systems. Gaseous hydrogen sulfide (H2S) levels are a key factor affecting the corrosion rate and these fluctuate due to the diurnal flow pattern of sewers. Currently, there is little known about how such fluctuations, in particular the periodic deprivation of H2S, may affect the corrosion activity. This study investigated the impact of the deprivation of H2S on the sulfide uptake rate (SUR) of concrete coupons incubated in laboratory corrosion chambers. After systematic evaluation of the gaseous H2S concentration profiles of two sewer systems, two types of profiles, i.e. short- (1 h) and long- (12 h) term deprivation of H2S, were applied to the concrete coupons. In comparison to the baseline SUR, exposing the concrete coupon to 0 ppm of H2S for 1 h consistently caused a temporary increase of the SUR (i.e. 3.2%-12.5%) following re-supply of H2S at baseline levels. With the continuous re-supply of H2S, there was gradual and steady decrease of SUR to the level close to the baseline SUR. However, for the case after deprivation of H2S for 12 h, the SUR was 5.1% lower than baseline SUR and gradually increased to a level similar to the baseline SUR during the 20 -30 min of continuous re-supply of H2S. In addition, the simultaneous deprivation of H2S and O-2 for 1 h had negligible impact on the SUR Further analysis suggests that the historically accumulated intermediates of sulfide oxidation could act as electron donors for sulfide oxidizing bacteria (SOB). The replenishment of the intermediates upon the re-supply of H2S could play a key role in the increase of SUR after short-term deprivation of H2S. However, the activity of SOB could be diminished after long-term deprivation of H2S, although the sulfur intermediates still could be available. Estimating the sulfide uptake by concrete using the SUR of the average H2S concentration could lead to overestimation of the sulfide uptake. There could be more significant overestimation for the case with longer deprivation of H2S. (C) 2019 Published by Elsevier Ltd.

KeywordSewer Concrete corrosion Sulfide Fluctuation Uptake
DOI10.1016/j.watres.2019.03.074
Funding OrganizationAustralian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; 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Indexed BySCI
Language英语
Funding ProjectAustralian Research Council[LP0882016] ; Australian water industry[LP0882016] ; University of Queensland ; Chinese Scholarship Council ; Queensland State Government's Early Career Accelerate Fellowship ; Australian Research Council DECRA Fellowship[DE170100694]
WOS Research AreaEngineering ; Environmental Sciences & Ecology ; Water Resources
WOS SubjectEngineering, Environmental ; Environmental Sciences ; Water Resources
WOS IDWOS:000468253500045
WOS KeywordMICROBIAL CORROSION ; OXIDIZING BACTERIA ; CORRODING CONCRETE ; RELATIVE-HUMIDITY ; OXIDATION ; TEMPERATURE
PublisherPERGAMON-ELSEVIER SCIENCE LTD
Funding OrganizationAustralian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; Australian water industry ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; University of Queensland ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Chinese Scholarship Council ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Queensland State Government's Early Career Accelerate Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; Australian Research Council ; 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Queensland State Government's Early Career Accelerate Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship ; Australian Research Council DECRA Fellowship
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ihb.ac.cn/handle/342005/28110
Collection水环境工程研究中心
Corresponding AuthorKeller, Jurg
Affiliation1.Univ Queensland, Adv Water Management Ctr, Brisbane, Qld 4072, Australia
2.Univ Wollongong, Sch Civil Min & Environm Engn, Wollongong, NSW 2522, Australia
3.Chinese Acad Sci, Inst Hydrobiol, Wuhan 430072, Hubei, Peoples R China
Recommended Citation
GB/T 7714
Sun, Xiaoyan,Jiang, Guangming,Bond, Philip L.,et al. Periodic deprivation of gaseous hydrogen sulfide affects the activity of the concrete corrosion layer in sewers[J]. WATER RESEARCH,2019,157(1):463-471.
APA Sun, Xiaoyan,Jiang, Guangming,Bond, Philip L.,&Keller, Jurg.(2019).Periodic deprivation of gaseous hydrogen sulfide affects the activity of the concrete corrosion layer in sewers.WATER RESEARCH,157(1),463-471.
MLA Sun, Xiaoyan,et al."Periodic deprivation of gaseous hydrogen sulfide affects the activity of the concrete corrosion layer in sewers".WATER RESEARCH 157.1(2019):463-471.
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